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朱文帅

教授,博导
E-mail: zhuws(AT) ujs(DOT)edu(DOT) cn

 

朱文帅, 男,教授,博导, 国家优秀青年科学基金

 

个人学习和工作经历:

20175至今  365.com,教授,博士生导师

201412—20174  365.com,副教授,博士生导师

20151—20169   橡树岭国家实验室访问学者(美国)

20128—201411 365.com,副教授,硕士生导师

20097—20127 365.com,讲师

20097—201112 江苏大学动力工程及工程热物理学科博士后

20069—20096 江苏大学环境学院 (博士)

20039—20066 365.com/西华师范大学化学化工学院 (硕士)

19989—20026 淮阴师范学院化学系 (本科)

 

研究方向:

1. 绿色化工:基于石油化工领域的汽、柴油超深度脱硫,着重新型催化剂、吸附剂的设计和清洁生产工艺研究。

2. 新型化工材料制备:二维层状材料、介孔材料、新型离子液体设计制备及其在能源领域的应用。

3. 环境保护化学:新型吸附剂设计及去除环境中持久性性有机污染物,研究污染控制技术中的化学问题。

 

5年的学术成就:

科研工作涉及石油化工、绿色化学和环境催化等领域,近年来主要从事新型催化剂和吸附剂的设计及其用于汽、柴油超深度脱硫的研究工作,先后主持和参与了多项国家自然科学基金、国家博士后科学基金、江苏省自然科学基金等课题,共计发表研究论文110余篇,其中SCI收录论文90余篇。近些年工作发表在Nature Commun., Angew. Chem. Int. Ed., AIChE J., Small, Chem. Commun., Green Chem., ChemSusChem., Europ. Chem. J., Chem. Eng. J., Ind. Eng. Chem. Res. 等期刊,被引用3000余次。

 

课题项目:

在研项目

1.  国家自然科学基金优秀青年科学基金21722604),130万,2018.1-2020.12

2.  国家自然科学基金面上(21576122),65万,2016.1-2019.12

3. 江苏省六大人才高峰JNHB-004), 2015.1-2017.12

结题项目:

1. 国家自然科学基金(211060552012.1-2014.12

2. 江苏省自然科学基金(BK20115062011.7-2014.6

3. 中国博士后科学基金特别资助(No. 2010035562010.7-2011.12

 

专利:

1.  离子液体萃取-催化氧化脱硫的方法,200710133235.8(授权)

2.  一种利用FeCl3离子液体萃取-催化氧化脱硫的方法,200910030020.2(授权)

3.  一种磁性离子液体及其制备方法和用途,201210381746.2(授权)

4.   一种多酸类化合物和制备方法及在氧化燃油脱硫中的用途,201210381772.5(授权)

5.  一种介孔硅材料及其制备方法和应用,201310399683.8(授权)

6. 一种含高分散性钨的介孔材料及其制备方法和应用,201310399805.3(授权)

7. 一种光氧化脱除燃油中硫化物的方法,201410342715.5(授权)

8.  一种类石墨烯型氮化硼负载离子液体催化剂制备方法及其应用,201410040820.3(授权)

9.  一种哌啶类离子液体催化氧化燃油脱硫的方法,201410010392.X(授权)

10.  一种离子液体催化氧化燃油脱硫的方法,201410231387.1(授权)

11.  一种有序的含有金属活性中心的介孔材料及其应用,201410051166.6

12.  一种少层氮化硼及其制备方法和应用,201410334628.5

13. 一种利用液氮气化制备二维六方氮化硼纳米片的方法, 201610454689.4

14. 一种质子型离子液体的制备方法及其用途,201610126455.7

15. 一种超疏水聚苯乙烯/氮化碳复合薄膜及其制备方法,201410630900.4

16. 一种利用蒸发溶剂引导晶面控制合成高比表面积六方氮化硼的工艺,201510616527.1

17. 类石墨烯型氮化硼负载磷钨酸催化剂及其制备方法和应用,201510702034.X

18. 层状氮化硼的层间限域铜纳米颗粒的催化剂及其制备方法与应用,201610260117.2

19. 一种含钨介孔二氧化钛微球及其制备方法和应用,201610208143.0

20. 一种负载型杂多酸离子液体及其制备方法和应用,201610208011.8

 

部分发表论文:

[1] Wenshuai Zhu, Zili Wu, Foo Guo Shiou, Xiang Gao, Mingxia Zhou, Bin Liu, Veith Gabriel M., Peiwen Wu, Browning Katie L., Lee Ho Nyung,  Huaming Li, Sheng Dai*, Huiyuan Zhu*, Taming interfacial electronic properties of Pt nanoparticles on vacancy-abundant boron nitride nanosheets for enhanced catalysis, Nature Commun., 2017, 8, 15291.

[2] Wenshuai Zhu*, Xiang Gao, Qian Li, Hongping Li, Yanhong Chao, Meijun Li, Shannon M. Mahurin, Huaming Li, Huiyuan Zhu*, Sheng Dai*, Controlled Gas Exfoliation of Boron Nitride into Few-Layered Nanosheets, Angew. Chem. Int. Ed., 2016, 55(36): 10766–10770.

[3] Hongping Li, Yonghui Chang, Wenshuai Zhu*, Siwen Zhu, Wei Jiang, Ming Zhang, Jiexiang Xia, Huaming Li*, The selectivity for sulfur removal from oils: an insight from conceptual density functional theory, AIChE J., 2016, 62(6):2087-2100.

[4] Jun Xiong, Huaming Li*, Lei Yang, Jing Luo, Yanhong Chao, Jingyu Pang, Wenshuai Zhu*, Metal-free boron nitride adsorbent for ultra-deep desulfurization, AIChE J., 2017, DOI: 10.1002/aic.15695.

[5] Jun Xiong, Wenshuai Zhu, Huaming Lia, Yehai Xu, Wei Jiang, Suhang Xun, Hui Liu, Zhen Zhao, Immobilized Fenton-like ionic liquid: catalytic performance for oxidative desulfurization, AIChE J., 2013, 12(59), 4696–4704.

[6] Mingtao Li, Wenshuai Zhu*, Pengfei Zhang, Yanhong Chao, Qian He, Bolun Yang, Huaming Li, Albinab Borisevich, Sheng Dai*, Graphene-analogues boron nitride nanosheets confining ionic liquids: a high performance quasi liquid solid electrolyte, Small, 2016,12(26): 3535–3542.

[7] Peiwen Wu, Wenshuai Zhu*, Yanhong Chao, Jinshui Zhang, Pengfei Zhang, Huiyuan Zhu, Changfeng Li, Zhigang Chen, Huaming Li*, Sheng Dai*, A Template- free solvent-mediated synthesis of high surface area boron nitride nanosheets for aerobic oxidative desulfurization, Chem. Commnun., 2016, 52, 144-147. (入选ESI高被引论文)

[8] Jun Xiong, Lei Yang, Yanhong Chao, Jingyu Pang, Peiwen Wu, Ming Zhang, Wenshuai Zhu*, Huaming Li*, A large number of low coordinated atoms in boron nitride for outstanding adsorptive desulfurization performance, Green Chem., 2016, 18, 3040-3047.

[9] Jun Xiong, Lei Yang, Yanhong Chao, Jingyu Pang, Ming Zhang, Wenshuai Zhu*, Huaming Li*, Boron nitride mesoporous nanowires with doped oxygen atoms for the remarkable adsorption desulfurization performance from fuels, ACS Sustain. Chem. Eng., 2016, 4 (8): 4457–4464.

[10] Suhang Xun, Wenshuai Zhu*, Yonghui Chang, Hongping Li, Ming Zhang, Wei Jiang, Dan Zheng, Yuejiao Qin, Huaming Li*, Synthesis of supported SiW12O40- based ionic liquid catalyst induced solvent-free oxidative deep-desulfurization of fuels, Chem. Eng. J., 2016, 288, 608–617.

[11] Peiwen Wu, Wenshuai Zhu*, Bilian Dai, Yanhong Chao, Changfeng Li, Hongping Li, Ming Zhang, Wei Jiang, Huaming Li, Copper nanoparticles advance electron mobility of graphene-like boron nitride for enhanced aerobic oxidative desulfurization, Chem. Eng. J., 2016, 301, 123–131.

[12] Wenshuai Zhu*, Chao Wang, Hongping Li, Peiwen Wu, Suhang Xun, Wei Jiang, Zhigang Chen, Zhen Zhao and Huaming Li*, One-pot extraction combined with metal-free photochemical aerobic oxidative desulfurization in deep eutectic solvent, Green Chem., 2015, 17 (4), 2464 – 2472. (入选ESI高被引论文)

[13] Jun Xiong, Wenshuai Zhu*, Hongping Li, Wenjing Ding, Yanhong Chao, Peiwen Wu, Suhang Xun, Ming Zhang, Huaming Li*, Graphene-like Boron Nitride Induced Remarkable Adsorption Capacity for Dibenzothiophene in Fuels, Green Chem., 2015, 17, 1647–1656. (入选ESI高被引论文)

[14] Jun Xiong, Wenshuai Zhu,*, Hongping Li, Wenjing Ding, Yanhong Chao, Peiwen Wu, Suhang Xun, Ming Zhang, Huaming Li*, Carbon doped Graphene-like Boron Nitride Induced Remarkable Adsorption Capacity for Dibenzothiophene in Fuels, J. Mater. Chem. A, 2015, 3, 12738 - 12747.

[15] Wenshuai Zhu*, Bilian Dai, Peiwen Wu, Yanhong Chao, Jun Xiong, Suhang Xun, Hongping Li, Huaming Li*, Graphene-analogue hexagonal BN supported with tungsten-based ionic liquid for oxidative desulfurization of fuels, ACS Sustain. Chem. Eng. 2015, 3, 186–194. (入选ESI高被引论文)

[16] Wenshuai Zhu*, Aimin Wei, Bilian Dai, Yanhong Chao, Changfeng Li, Huaming Li*, Sheng Dai*, Controllable fabrication of tungsten oxide nanoparticles confined in graphene-analogous boron nitride as an efficient desulfurization catalyst, Chem. A Europ. J., 2015, 21(43): 15421–15427.

[17] Wenjing Ding, Wenshuai Zhu*, Jun Xiong, Lei Yang, Aimin Wei, Ming Zhang, Hui Liu, Huaming Li*, Novel heterogeneous iron-based redox ionic liquid supported on SBA-15 for deep oxidative desulfurization of fuels, Chem. Eng. J., 2015, 266, 213–221. (入选ESI高被引论文)

[18]Dan Zheng, Wenshuai Zhu*, Suhang Xun, Miaomiao Zhou, Ming Zhang, Wei Jiang, Yuejiao Qin, Huaming Li*, Deep oxidative desulfurization of dibenzothiophene using low-temperature-mediated titanium dioxide catalyst in ionic liquids, Fuel, 2015, 159, 446-453. (入选ESI高被引论文)

[19] Wei Jiang, Wenshuai Zhu*, Hongping Li , Xin Wang, ShengYin, Yonghui Chang, Huaming Li*, Temperature-responsive ionic liquid extraction and separation of the aromatic sulfur compounds, Fuel, 2015, 140, 590–596. (入选ESI高被引论文)

[20] Suhang Xun, Wenshuai Zhu*, Yonghui Chang, Hongping Li, Ming Zhang, Wei Jiang, Dan Zheng, Yuejiao Qin, Huaming Li*, Synthesis of supported SiW12O40- based ionic liquid catalyst induced solvent-free oxidative deep-desulfurization of fuels, Chem. Eng. J., 2016, 288, 608–617.

[21] Wei Jiang, Wenshuai Zhu*, Yonghui Chang , Yanhong Chao, Sheng Yin, Hui Liu, Fengxia Zhu, Huaming Li*, Ionic liquid extraction and catalytic oxidation desulfurization of fuels using dialkylpiperidinium tetrachloroferrates catalysts, Chem. Eng. J., 2014, 250, 48–54.

[22] Ming Zhang, Wenshuai Zhu*, Huaming Li*, Suhang Xun, Wenjing Ding, Jianjun Liu, Zhen Zhao, One-pot synthesis, characterization and desulfurization of functional mesoporous W-MCM-41 from POM-based ionic liquids, Chem. Eng. J., 2014, 243 386–393.

[23] Yanhong Chao, Wenshuai Zhu*, Xiangyang Wu, Fangfang Hou, Suhang Xun, Peiwen Wu, Haiyan Ji, Hui Xu, Huaming Li*, Application of graphene-like layered molybdenum disulfide and its excellent adsorption behavior for doxycycline antibiotic, Chem. Eng. J., 2014, 243, 60–67.

[24] QingQing Gu, Wenshuai Zhu*, Suhang Xun, Yonghui Chang, Jun Xiong , Ming Zhang, Wei Jiang, Fengxia Zhu, Huaming Li*, Preparation of highly dispersed tungsten species within mesoporous silica by ionic liquid and their enhanced catalytic activity for oxidative desulfurization, Fuel, 2014, 117, 667-673.

[25] Wei Jiang, Wenshuai Zhu*, Yonghui Chang, Huaming Li*, Yanhong Chao, Jun Xiong, Hui Liu, Fengxia Zhu, Oxidation of aromatic sulfur compounds catalyzed by organic hexacyanoferrates in ionic liquids with low concentration of H2O2 as oxidant, Energy Fuel, 2014, 28 (4), 2754–2760.

[26] Wenshuai Zhu, Peiwen Wu, Lei Yang, Yonghui Chang, Yanhong Chao, Huaming Li, Yunqing Jiang, Wei Jiang, Suhang Xun, Pyridinium-Based Temperature- responsive Magnetic Ionic Liquid for Oxidative Desulfurization of Fuels, Chem. Eng. J., 2013, 229, 250–256. (入选ESI高被引论文)

[27] Ming Zhang, Wenshuai Zhu, Huaming Li, Suhang Xun, Qingqing Gu, Zhen Zhao, Qian Wang, Deep oxidative desulfurization of dibenzothiophene with POM-based hybrid materials in ionic liquid, Chem. Eng. J., 2013, 220, 328–336. (入选ESI高被引论文)

[28] Wenshuai Zhu*, Peiwen Wu, Yanhong Chao, Huaming Li*, Fang Zou, Suhang Xun, Fengxia Zhu, Zhen Zhao, A Novel Reaction-Controlled Foam-Type Polyoxometalate Catalyst for Deep Oxidative Desulfurization of Fuels, Ind. Eng. Chem. Res., 2013, 52 (49), 17399– 17406.

[29] Wenshuai Zhu, Guopeng Zhu, Huaming Li, Yanhong Chao, Ming Zhang, Daolin Du, Qian Wang, Zhen ZhaoCatalytic Kinetics of Oxidative Desulfurization with Surfactant-type Polyoxometalate-based Ionic LiquidsFuel Process. Tech.2013, 106, 70–76.

[30] Yunqing Jiang, Wenshuai Zhu, Huaming Li, Sheng Yin, Hua Liu, Qingjie Xie, Oxidative desulfurization of fuels catalyzed by Fenton-Like ionic liquids at room temperature. ChemSusChem 2011, 4, 399-403.

[31] Yuxiao Ding, Wenshuai Zhu, Huaming Li, Wei Jiang, Ming Zhang, Yuqing Duan, Yonghui Chang, Catalytic oxidative desulfurization with hexatungstate/aqueous H2O2/ionic liquid emulsion system. Green Chem., 2011, 13, 1210–1216.

[32] Lining He, Huaming Li, Wenshuai Zhu, Junxiang Guo, Xue Jiang, Jidong Lu, Yongsheng Yan, Deep Oxidative Desulfurization of Fuels Using Peroxophospho- molybdate Catalysts in Ionic Liquids, Ind. Eng. Chem. Res., 2008, 47, 6890–6895.

[33] Huaming Li*, Wenshuai Zhu, Yan Wang, Jingtong Zhang, Jidong Lu, Yongsheng Yan. Deep oxidative desulfurization of fuels in redox ionic liquids based on iron chloride. Green Chem., 2009, 11, 810-815.

[34] Wangli Huang, Wenshuai Zhu, Huaming Li, Hua Shi, Guopeng Zhu, Hui Liu, Guangying Chen. Heteropolyanion-based ionic liquid for deep desulfurization of fuels in ionic liquids. Ind. Eng. Chem. Res., 2010, 49, 8998–9003.

[35] Wenshuai Zhu, Huaming Li, Xue Jiang, Yongsheng Yan, Jidong Lu, Lining He, Jiexiang Xia. Commercially available molybdic compound-catalyzed ultra-deepdesulfurization of fuels in ionic liquids. Green Chem., 2008, 10, 641–646.

[36] Wenshuai Zhu, Huaming Li, Xue Jiang, Yongsheng Yan, Jidong Lu, and Jiexiang Xia. Oxidative desulfurization of fuels catalyzed by peroxotungsten and peroxomolybdenum complexes in ionic liquids. Energy Fuels, 2007, 21(5): 2514-2516. (入选ESI高被引论文)

 

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